New Transparent, Ultra-Stretchable, Foldable Elastic OLED

Imagine an electronic display nearly as clear as a window, or a curtain that illuminates a room, or a smartphone screen that doubles in size, stretching like rubber. Now imagine all of these being made from the same material.

Organic light-emitting device: Schematic (left) and top-view (right) illustrations of an encapsulated fully stretchable OLED display comprising 5×5 pixels.

Researchers from UCLA's Henry Samueli School of Engineering and Applied Science have developed a transparent, elastic organic light-emitting device, or OLED, that could one day make all these possible. The OLED can be repeatedly stretched, folded and twisted at room temperature while still remaining lit and retaining its original shape.

OLED technology is used today in screens for many smartphones and some televisions. The new ultra-stretchable OLED material developed at UCLA could lead to foldable and expandable screens for new classes of smartphones and other personal electronic devices; electronics-integrated clothing; wallpaper-like lighting; new minimally invasive medical tools; and many other applications.

UCLA Engineering develops flexible and stretchable LEDs

"Our new material is the building block for fully stretchable electronics for consumer devices," said Qibing Pei, a UCLA professor of materials science and engineering and principal investigator on the research. "Along with the development of stretchable thin-film transistors, we believe that fully stretchable interactive OLED displays that are as thin as wallpaper will be achieved in the near future. And this will give creative electronics designers new dimensions to exploit."

The research is published online in the peer-reviewed journal Nature Photonics. The lead author of the study is Jiajie Liang, a postdoctoral scholar in Pei's Soft Materials Research Laboratory at UCLA.

The researchers stretched and restretched the OLED 1,000 times, extending it 30 percent beyond its original shape and size, and it still continued to work at a high efficiency. In another test to determine the material's maximum stretch, the researchers found it could be stretched to more than twice its original size while still functioning. In addition, it can be folded 180 degrees and can be twisted in multiple directions.

The material has a single layer of an electro-luminescent polymer blend sandwiched between a pair of new transparent elastic composite electrodes. These electrodes are made of a network of silver nanowires inlaid into a rubbery polymer, which allows the device to be used at room temperatures. All of these layers are fully stretchable, foldable and twistable. The new material can also be fabricated in a relatively simple all-solution–based process.

"The lack of suitable elastic transparent electrodes is one of the major obstacles to the fabrication of stretchable display," Liang said. "Our new transparent, elastic composite electrode has high visual transparency, good surface electrical conductivity, high stretchability and high surface smoothness — all features essential to the fabrication of the stretchable OLED."

The team also demonstrated this ultra-flexible OLED could contain multiple pixels, rather than just a solid block of light. This could pave the way for electronic displays comprising many thousands of pixels. They accomplished this by assembling the silver nanowire–based electrodes into a cross-hatched pattern, with one layer of columns and one layer of rows.

"While we perceive a bright future where information and lighting are provided in various thin, stretchable or conformable form factors, or are invisible when not needed, there are still major technical challenges," Pei said. "This includes how to seal these materials that are otherwise sensitive to air. Researchers around the world are racing the clock tackling the obstacles. We are confident that we will get there and introduce a number of cool products along the way."

Pei is also a member of the California NanoSystems Institute (CNSI) at UCLA.

Other authors of the study include Lu Li, a UCLA postdoctoral scholar; UCLA engineering graduate student Xiaofan Niu; and Zhibin Yu, a former UCLA doctoral student and postdoctoral scholar who is now a postdoctoral scholar at UC Berkeley.

The research was funded by the National Science Foundation and the Air Force Office of Scientific Research.

The UCLA Henry Samueli School of Engineering and Applied Science, established in 1945, offers 28 academic and professional degree programs and has an enrollment of more than 5,000 students. The school's distinguished faculty are leading research to address many of the critical challenges of the 21st century, including renewable energy, clean water, health care, wireless sensing and networking, and cyber-security. Ranked among the top 10 engineering schools at public universities nationwide, the school is home to eight multimillion-dollar interdisciplinary research centers in wireless sensor systems, wireless health, nanoelectronics, nanomedicine, renewable energy, customized computing, the smart grid, and the Internet, all funded by federal and private agencies and individual donors.

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